What is it about?
Two-dimensional optical spectroscopy probes the correlated motions of electrons and nuclei. This paints a very detailed picture of how a molecule behaves and responds when stimulated by light. We have developed mathematical algorithms that dissect these various components of motion out of the spectrum and build useful effective molecular models that can be analyzed and interpreted within other contexts.
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This page is a summary of: Coherent and dissipative quantum process tensor reconstructions in two-dimensional electronic spectroscopy, The Journal of Chemical Physics, April 2019, American Institute of Physics,
DOI: 10.1063/1.5082165.
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