What is it about?
The focus of the article then shifts to detailing the current state of research in the realm of anisotropic 2D material-based polarization-sensitive photodetectors. It provides a comprehensive description of the working principles behind polarization-sensitive photodetectors with different structural designs, shedding light on the underlying mechanisms that enable their polarization sensitivity.
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Why is it important?
In the natural world, polarized light is predominantly produced through the process of Rayleigh scattering that affects sunlight[Science Advances 2017]. Many species of insects are endowed with the ability to detect this polarized light, a capability facilitated by their compound eyes[Science Advances 2017, Current Biology 2019]. However, this sensory function is not shared by the human visual system. Despite this constraint, human creativity has ingeniously harnessed polarized light through photodetectors, transforming the polarization of light into electrical signals. This technological breakthrough enables us to uncover deeper understandings of the natural world, insights that would be out of reach for our senses alone. This review meticulously navigates from the structural nuances of anisotropic 2D materials to their detailed optical and electrical characterization, culminating in a comprehensive exploration of the various structural configurations of 2D material-based polarization-sensitive photodetectors. It is designed to foster a profounder comprehension of these photodetectors among researchers and to serve as a pivotal reference for the innovation and advancement of the next generation of such devices.
Perspectives
The study of polarization-sensitive photodetectors based on 2D materials has been a vibrant field, with continuous advancements in performance. Despite the progress, there are several frontiers that offer potential for significant breakthroughs in this domain. First, the majority of anisotropic 2D materials currently in use are limited to one or two elements. Ternary compounds are known for their intriguing anisotropic characteristics and present a largely untapped area of research. Expanding the exploration into ternary anisotropic 2D materials could be a promising avenue for future studies. Second, while theoretical calculations have been conducted on polarization-sensitive photodetectors through defects and doping methods, experimental validation is still in the infancy. Consequently, the experimental approach could be initiated in this direction, employing vacancy and doping techniques to modify the intrinsic anisotropy of 2D materials. This targeted manipulation holds the potential to significantly enhance the performance capabilities of photodetectors. Third, the heterojunction polarization-sensitive photodetectors that are currently prevalent often include an anisotropic 2D material as a component of the junction. While this simplifies much research challenges, it may also reduce the polarization ratio due to the inclusion of isotropic materials. Future research could benefit from developing heterojunction photodetectors that integrate multiple anisotropic 2D materials to maintain or even enhance anisotropy. Fourth, isotropic 2D materials have the potential to achieve polarization sensitivity by altering their morphological attributes or leveraging surface plasmon resonance to disrupt their in-plane absorption symmetry. Integrating these technologies could further refine the polarization sensitivity of photodetectors by breaking the inherent absorption symmetry of 2D materials. The current polarization-sensitive photodetectors that leverage anisotropic 2D materials are predominantly focused on the detection of linearly polarized light. The capability to sense circularly polarized light, which typically involves the use of chiral organic molecules or chiral structures, remains an area ripe for innovation. Moving forward, the development of anisotropic 2D material-based photodetectors should pivot toward embracing the detection of both circularly and partially polarized light. This strategic expansion will not only diversify the photodetector functional scope but also enhance their relevance and effectiveness in a multitude of scientific and technological applications.
Prof. Xianguang Yang
Jinan University
Read the Original
This page is a summary of: Structural and optoelectronic characterization of anisotropic two-dimensional materials and applications in polarization-sensitive photodetectors, Applied Physics Reviews, January 2025, American Institute of Physics,
DOI: 10.1063/5.0226193.
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